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程国林

2018-10-25  点击:[]

                                             程国林,

                                             教授/博导(2017)     

                                             应用化学系系主任(2021)

                                             福建省高层次人才C类(2021)

                                             福建省新世纪优秀人才(2017)

                                             福建省杰出青年人才培育计划(2015)

                                             厦门市重点人才(2017)

Group website:http:///www.x-mol.com/groups/glcheng

地址:厦门市集美大道668号泛华科技大楼 B612

邮箱glcheng@hqu.edu.cn


教育工作经历:

2011-2014-2017-今,讲师/副教授/教授,华侨大学,不限ip开户即送84元体验金

2014-2015,访学,The Scripps Research Institute (Jin-quan Yu 院士)

2007-2011,博士,清华大学, 化学系 (胡跃飞 教授)

2005-2007,硕士,浙江大学, 材化学院 (戴立言 教授)

2001-2005,本科,东北石油大学, 化学化工学院

研究兴趣:

羰基与亚胺化学;碳碳键断裂与重组;药物中间体的合成

科研基金

3) 2021-2024 国家自然科学基金面上项目 (22071068),在研

2) 2017-2020 国家自然科学基金面上项目 (21672075)已结题

1) 2013-2015 国家自然科学基金青年项目 (21202048),已结题

课题组成员:

2023年计划招生硕士生2-3名,博士生1-2名。

2021级 黎志勇、樊婧雯、郭海琳、丁宇浩;2020级 张雨青;2019级 田青于;2018级 陈燕惠2017级 文思

已毕业博士

2018级 巴聃(三峡大学);2016级 吕薇薇(阜阳师范大学两次国奖);2013级 翁云翔(清华大学博/福师大副教授

已毕业硕士

2018级 赵泽民;2017级 刘景2016级 余佳(国奖)、葛百潞2015级 肖上运;2014级 朱瑞丰(国奖)、薛露露

学术奖励:

福建省自然科学奖三等奖 (2019,第2)

第十二届福建省自然科学优秀学术论文二等奖(2016,第1)

发表论文:

迄今在SCI主流杂志发表论文70余篇(J. Am. Chem. Soc. 3篇;Angew. Chem. Int. Ed. 3篇;Nat. Commun. 1篇;ACS Catal. 1篇)。

71. Wen S.; Zhang, Y.; Tian, Q.; Chen, Y.; Cheng, G.* Ruthenium(II)-Catalyzed Synthesis of CF3-isoquinolinones via C−H Activation/Annulation of Benzoic Acids and CF3-Imidoyl Sulfoxonium Ylides. submitted


70. Ba,D.; Wen, S.; Tian, Q.; Chen, Y.; Cheng, G.* Blue Light Induced Insertion of Carbene into C(CO)-C Bonds of 1,3-Diones. Chin. J. Org. Chem. 2022, Revised


69. Yu, J.; Wen S.; Tian, Q.; Chen, Y.; Cheng, G.* Rhodium(I)-Catalyzed Regioselective C−H Alkenylation of 2,2′-Bipyridine Derivatives with Alkynes

Synthesis 2022, invited Feature article. Aceepted.

[Link]

68. Wen, S.;Chen, Y.; Tian, Q.;Zhang, Y.;Cheng, G.*Transition Metal-, Additive-, and Solvent-free [3+3] Annulation of CF3-Imidoyl Sulfoxonium Ylides with Cyclopropenones to Give Multifunctionalized CF3-Pyridones. J. Org.Chem.2022, 87, 1124-1132 .

[Link]

67. Chen, Y.; Wen S.; Tian, Q.; Zhang, Y.; Cheng, G.* Transition Metal-Free C–H Thiolation via Sulfonium Salts using β-Sulfinylesters as the Sulfur Source.

Org. Lett. 2021, 23, 7905–7909.

[Link]


66. Wen S.; Tian, Q.; Chen, Y.; Zhang, Y.; Cheng, G.* Annulation of CF3-Imidoyl Sulfoxonium Ylides with 1,3-Dicarbonyl Compounds: Access to 1,2,3-Trisubstituted-5-trifluoromethylpyrroles.Org. Lett. 2021, 23,  7407–7411.

[Link]


65. Zhao, Z.; Tian, Q.; Chen, Y.; Wen S.; Zhang, Y.; Cheng, G.*Based-Promoted Stereoselective Hydrogenation of Ynamides with Sulfonyl Hydrazide to Give Z-Enamides. J. Org.Chem.2021, 86, 10407-10413 .

[Link]


64. Tian, Q.; Xiao, S.;  Cheng, G.* Base-Promoted Synthesis of 3-Alkenyl-2-pyridonesfromN-Propargyl-β-enaminones and Aryl Aldehydes. Chin. J. Chem. 2021, 39, 2781-2788. 

[Link]


63.Yang, M.; Wang, J.; Lv, W.; Ba, D.;   Cheng, G.*; Wang, L.*Synthesis of 2-alkenyl-4H-3,1-benzoxazin-4-ones through HFIP-mediated decarboxylative [4+2]-annulation of isatoic anhydrides with cyclopropenones under silver catalysis.Adv. Synth. Catal.2021, 363, 4085-4090

[Link]


62. Wang, J.; Ba, D.;  Yang, M.;Cheng, G.*; Wang, L.*Regioselective Synthesis of 2,4-Diaryl-6-trifluoromethylated Pyridines through Copper-Catalyzed Cyclization of CF3‑Ynones and Vinyl Azides. J. Org.Chem.2021,86, 6423-6432.

[Link]



61. Chen, Y.; Lv, W.; Ba, D.; Wen S.; Cheng, G.* Palladium-Catalyzed Chemoselective Synthesis of 2-Aminocinnamyl Esters via Sequential Amination and Olefination of Aryl Iodides. J. Org. Chem. 2020,  85, 13280-13289.

[Link]


60.Lv, W.;  Liu S.; Chen, Y.; Wen S.; Lan Y.;* Cheng, G.* Palladium-Catalyzed Intermolecular trans-Selective Carbofunctionalization of Internal Alkynes to Highly Functionalized Alkenes. ACS. Catal. 2020, 10, 10516–10522.

[Link]


Highlighted by Synfacts:  https://doi.org/10.1055/s-0040-1706339

Highlighted by X-Mol: https://www.x-mol.com/news/466165



59. Zeng L.; Xu J.; Zhang D.; Yan Zh.; Cheng G.; Rao W.; Gao L.Catalytic Enantioselective [2+2] Cycloaddition of α-Halo Acroleins: Construction of Cyclobutanes Containing Two Tetrasubstituted Stereocenters. Angew. Chem., Int. Ed. 2020, 59, 21890-21894. 

[Link]


58. Lv, W.;  Chen, Y.; Wen S.; Ba, D.;  Cheng, G.* Modular and Stereoselective Synthesis of C-Aryl Glycosides via Catellani Reaction. J. Am. Chem. Soc. 2020, 142, 14864–14870. 

[Link]


Highlighted by Synfacts:  https://doi.org/10.1055/s-0040-1706330

Highlighted by X-Mol: https://www.x-mol.com/news/463918


57. Ba, D.; Wen S.; Chen, Y.; Lv, W.; Cheng, G.*Rhodium(II)-catalyzed multicomponent assembly of α,α,α-trisubstituted esters via formal insertion of O–C(sp3)–C(sp2) into C–C bonds. Nat. Commun. 202011, 4219

[Link]



Highlighted by Synfacts:  https://doi.org/10.1055/s-0040-1706341

Highlighted by X-Mol: https://www.x-mol.com/news/466051

 

56. Liu J. Ba, D.; Chen, Y.; Wen S.;  Cheng, G.* Tandem reaction to 3-(2-quinolyl) chromones from ynones and quinoline N-oxides under transition metal- and additive-free conditions. Chem. Commun., 2020, 56,  4078-4081

[Link]


55. Wen S.; Chen, Y.; Ba, D.; Lv, W.; Cheng, G.* Ruthenium(II)-Catalyzed Construction of Isocoumarins via Dual C−H/C−C Activation of Sulfoxonium Ylides. J. Org. Chem. 2020, 85, 1216-1223. 




54. Ge, B; Peng, Y.; Liu, J.; Wen S.; Peng, C.; Cheng, G.* Acid-Promoted Cleavage of the C−C Double Bond of N-(2-Hydroxylphenyl)enaminones for the Synthesis of Benzoxazoles. Tetrahedron. 2020, 76, 130818-130825. 

[Link]



53. Liu, J.; Ba, D.; Lv, W.; Chen, Y.; Zhao, Z.; Cheng, G.* Based-promoted Michael addition/Smiles rearrangement/N-arylation cascade:One-step syntheses of 1,2,3-trisubstituted 4-quinolones from ynones and sulfonamides. Adv. Synth. Catal. 2020, 362, 213-223.

[Link]



52. Ba, D.; Chen, Y.; Lv, W.; Chen, Y.; Wen S.; Cheng, G.* Copper-Catalyzed Three-Component Cascade Michael Addition/Heck-Type Alkylation/Annulation: Accessing Fully Substituted 1,3-Dihydro-2H-pyrrol-2-ones. Org. Lett. 201921, 8603-8606.

[Link]



51. Lv, W.; Chen, Y.; Zhao, Z.; Wen, S.; Cheng, G.* Palladium-Catalyzed Regioselective Heck Coupling of Alkynes with Aryl Iodides for the Synthesis of Trisubstituted Allenes.  Org. Lett. 2019, 21, 7795-7798

[Link]

50. Wen S.; Lv, W.; Ba, D.; Liu, J.; Cheng, G.* Ruthenium(II)-catalyzed chemoselective deacylative annulation of 1,3-diones with sulfoxonium ylides via C–C bond activation. Chem. Sci. 2019, 109104-9108

[Link]



49. Yu, J.; Wen, S.; Ba, D.; Lv, W.;  Chen, Y. Cheng, G.* Rhodium(III)-Catalyzed Site-Selective C−H Acylmethylation of 2,2′-Bipyridine-6-carboxamides with Sulfoxonium Ylides.  Org. Lett. 2019,  21, 6366-6369

[Link]



48. Lv, W.; Wen, S.; Liu, J.;  Cheng, G.* Palladium-Catalyzed Ortho- C−H Methylation of Benzoic Acids. J. Org. Chem. 2019, 84, 9786-9791.

[Link]


47. Lv, W.; Yu, J.; Ge, B.; Wen, S.; Cheng, G.* Palladium-Catalyzed Catellani-Type bis-Silylation and bis-Germanylation of Aryl Iodides and Norbornenes. J. Org. Chem. 2018, 83,12683-12693.

[Link]


 

                 

 

46. Ge, B.; Lv W.; Yu J.; Xiao S.; Cheng G.* Base-promoted C–C bond cleavage for the synthesis of 2,3,4-trisubstituted pyrroles from N-propargyl β-enaminones. Org. Chem. Front. 2018, 5, 3103-3107.

[Link]


 

                 

45. Cheng, G;* Lv, W.; Xue, L. Base-promoted ring-closing carbonyl–allene metathesis for the synthesis of 2,4-disubstituted pyrroles. Green Chem. 2018, 20, 4414-4417  selected as back cover. 

[Link]


  

44. Lv, W.; Wen, S.; Yu, J.; Cheng, G.* Palladium-Catalyzed Ortho-Silylation of Aryl Iodides with Concomitant Arylsilylation of Oxanorbornadiene: Accessing Functionalized (Z)-β-Substituted Vinylsilanes and Their Analogues. Org. Lett. 2018, 20, 4984-4987

[Link]


                 

43. Yu, J.; Lv, W.; Cheng, G.* Palladium-Catalyzed Site-Selective C−H Arylation of 2,2′-Bipyridine-6-carboxamides via a Rollover Cyclometalation Pathway. Org. Lett. 2018, 20, 4762-4735.

[Link]


 

                 

42. Zhang,H.; Shen,J.; Cheng,G.; Wu,B.; Cui, X.* Base-Promoted Synthesis of 2,4,6-Triarylpyridines from Enaminones and Chalcones. Asian J. Org. Chem. 2018, 7, 1089 – 1092. 

[Link]

                 

41. Weng, Y.; Kuai, C.;  Lv, W.; Cheng, G.* Synthesis of 2-Aminopyridines via a Base-Promoted Cascade Reaction of N-Propargyl Enaminones with Formamides. J. Org. Chem. 2018,83, 5002−5008. 

[Link]


 

  

40. Weng, Y.; Lv, W.; Yu, J.; Ge, B.; Cheng, G.* Preparation of 2,4,5-Trisubstituted Oxazoles through Iodine-Mediated Aerobic Oxidative Cyclization of Enaminones. Org. Lett. 2018, 20, 1853–1856. 

[Link]


                 

39. Cheng, G.*; Lv, W.; Kuai C.; Wen S; Xiao S. Base-Promoted Amide Synthesis from Aliphatic Amines and Ynones as Acylation Agents through C–C Bond Cleavage. Chem. Commun., 2018, 54, 1726-1729. 

[Link]


                 

 

Highlighted by Synfacts:  https://doi.org/10.1055/s-0037-1609138

 

38. Zhang H.; Shen J.; Cheng G.; Feng Y.; Cui X. One-Pot Synthesis of Benzo[b][1,4]oxazins via Intramolecular Trapping Iminoenol, Org. Lett. 2018, 20, 664-667

[Link]


 

                  

37. Xue, L.; Cheng, G.*;  Zhu, R.; Cui, X. *, Acid-Promoted Oxidative Methylenation of 1,3-DicarbonylCompounds with DMSO: Application to the Three-Component Synthesis of Hantzsch-TypePyridines. RSC Adv., 2017, 7, 44009-44012.

[Link]


 

 

36. Cheng, G.*; Xue, L.; Weng, Y.; Cui, X. *, Transition-Metal-Free Cascade Approach toward 2‑Alkoxy/2-Sulfenylpyridines and Dihydrofuro[2,3‑b]pyridines by Trapping In Situ Generated 1,4-Oxazepine. J. Org. Chem. 2017,  82, 9515-9524.

[Link]


                 

35. Cheng, G.;+ Wang P.; + Yu, J.-Q.*, Meta-CH Arylation and Alkylation of Benzylsulfonamide Enabled by a Pd(II)/Isoquinoline Catalyst. Angew. Chem., Int. Ed. 2017, 56, 8183-8186

[Link]

                 


34. Ding, Q.; Ye, S.; Cheng, G.; Wang, P.; Farmer, M. E.; Yu, J.-Q.*, Ligand-Enabled meta-Selective C–H Arylation of Nosyl-Protected Phenethylamines, Benzylamines, and 2-Aryl Anilines J. Am. Chem. Soc.2017, 139, 417-425

[Link]


                  

33. Zhu, R.; Cheng, G.*; Jia, C.; Xue, L.; Cui, X.*, Access to C4-Functionalized Quinolines via Copper-Catalyzed Tandem Annulation of Alkynyl Imines with Diazo Compounds. J. Org. Chem. 2016, 81, 7539-7544. 

[Link]


                 

32. Shen, J. H.; Yang, X. F.; Wang, F. Y.; Wang, Y.; Cheng, G.; Cui, X. L.*, Base-mediated regiospecific cascade synthesis of N-(2-pyridyl)pyrroles from N-propargylic beta-enaminones. Rsc Adv. 2016, 6,48905-48909. 

[Link]


                   

31. Shen, J. H.; Xue, L. L.; Lin, X.; Cheng, G.; Cui, X.*, The base-promoted synthesis of multisubstituted benzo b 1,4 oxazepines. Chem. Commun. 2016, 52, 3292-3295. 

[Link]


                 

30. Shen, J. H.; Wang, X. D.; Lin, X.; Yang, Z. H.; Cheng, G.; Cui, X.*, One-Pot Regiospecific Synthesis of Quinoxalines via a CH2-Extrusion Reaction. Org. Lett. 2016,18 , 1378-1381

[Link]


                 

29. Cheng, G.; Li, T.-J.; Yu, J.-Q.*, Practical Pd(II)-Catalyzed C-H Alkylation with Epoxides: One-Step Syntheses of 3,4-Dihydroisocoumarins. J. Am. Chem. Soc. 2015,137, 10950-10953

[Link]


 

                

28. Wang, F.; Shen, J.; Cheng, G.; Cui, X.*, Practical access to 1,3,5-triarylbenzenes from chalcones and DMSO. RSC Adv. 2015,5, 73180-73183. 

[Link]


                   

27. Shen, J.; Cai, D.; Kuai, C.; Liu, Y.; Wei, M. e.; Cheng, G.; Cui, X.*, Base-Promoted beta-C(sp(3))-H Functionalization of Enaminones: An Approach to Polysubstituted Pyridines. J. Org. Chem. 2015,80, 6584-6589.

[Link]


                   

26. Feng, Y.; Li, Y.; Cheng, G.; Wang, L.; Cui, X.*, Copper-Catalyzed Synthesis of 2-Arylquinazolinones from 2-Arylindoles with Amines or Ammoniums. J. Org. Chem. 2015,80, 7099-7107. 

[Link]


                   

25. Cheng, G.*; Weng, Y.; Yang, X.; Cui, X.*, Base-Promoted N-Pyridylation of Heteroarenes Using N-Propargyl Enaminones as Equivalents of Pyridine Scaffolds. Org. Lett. 2015,17, 3790-3793.

[Link]


 

 

 

24. Yang, X.; Cheng, G.*; Shen, J.; Kuai, C.; Cui, X.*, Cleavage of the C-C triple bond of ketoalkynes: synthesis of 4(3H)-quinazolinones. Org. Chem.Front. 2015,2, 366-368.

[Link]



                 

23. Wang, X.; Cheng, G.; Shen, J.; Yang, X.; Wei, M.-e.; Feng, Y.; Cui, X.*, A metal-free synthesis of diaryl-1,2-diketones by C-C triple bond cleavage of alkynones. Org. Chem.Front. 2014,1, 1001-1004. 

[Link]

     

                 

22. Cheng, G.; Zhang, H.; Cui, X., Copper(I)-catalyzed homo-coupling of terminal alkynes at room temperature under solvent and base free conditions using O2 as an oxidant. RSC Adv. 2014, 4, 1849-1852. 

[Link]

         

                   

21. Cheng, G.; Zeng, X.; Cui, X., Benzoquinone-Promoted Aerobic Oxidative Hydroxylation of Arylboronic Acids in Water. Synthesis. 2014, 295-300. 

[Link]

    

 

 

20. Li, P.; Cheng, G.*; Zhang, H.; Xu, X.; Gao, J.; Cui, X.*, Copper-Catalyzed One-Pot Synthesis of Unsymmetrical Arylurea Derivatives via Tandem Reaction of Diaryliodonium Salts with N-Arylcyanamide.J. Org. Chem. 2014, 79, 8156-8162. 

[Link]


 

                   

19. Feng, Y.; Zhang, H.; Cheng, G.*; Cui, X.,Synthesis of Indole Derivatives via Domino Reactions.Chin. J. Org. Chem. 2014, 34, 1499-1508. 

[Link]


                 

18. Wang, X.; Cheng, G.; Cui, X., Tandem synthesis of 3-allyl-chromones from alkynones and allylic alcohols under metal-free conditions. Chem. Commun. 2014, 50, 652-654

[Link]


                   

17. Gao, Y.; Song, Q.; Cheng, G.; Cui, X.,KI-catalyzed arylation of benzothiazoles from the coupling of aryl aldehydes with benzothiazoles in neat water. Org. Biom. Chem. 2014, 12, 1044-1047.

[Link]


 

 

16. Cheng, G.; Zeng, X.; Shen, J.; Wang, X.; Cui, X., A metal-free multicomponent cascade reaction for the regiospecific synthesis of 1,5-disubstituted 1,2,3-triazoles. Angew. Chem., Int. Ed. 2013, 52, 13265-13268

[Link]

                                       

                   

15. Shen, J.; Cheng, G.; Cui, X., "One pot" regiospecific synthesis of polysubstituted pyrroles from benzylamines and ynones under metal free conditions. Chem. Commun. 2013, 49, 10641-10643.

[Link]

 

 

           

14. Shao, C.; Zhang, Q.; Cheng, G.; Cheng, C.; Wang, X.; Hu, Y., Copper(I) Acetate-Catalyzed Cycloaddition between Azomethine Imines and Propiolates under Additive-Free Conditions. Eur. J. Org. Chem. 2013, 6443-6448.

[Link]


13. Cheng, G.; Cui, X., Efficient Approach to 4-Sulfonamidoquinolines via Copper(I)-Catalyzed Cascade Reaction of Sulfonyl Azides with Alkynyl Imines. Org. Lett. 2013, 15, 1480-1483.

[Link]

      

12. Zeng, X.; Cheng, G.; Shen, J.; Cui, X., Palladium-Catalyzed Oxidative Cross Coupling of N-Tosylhydrazones with Indoles: Synthesis of N-Vinylindoles. Org. Lett. 2013, 15, 3022-3025.         

[Link]

                     

11. Cheng, G.; Wang, X.; Bao, H.; Cheng, C.; Liu, N.; Hu, Y., Total Syntheses of (-)-Hanishin, (-)-Longmide B, and (-)-Longmide B Methyl Ester via a Novel Preparation of N-Substituted Pyrrole-2-Carboxylates. Org. Lett. 2012, 14, 1062-1065

[Link]


 

10. Shen, J.; Cheng, G.; Cui, X., Domino Reactions Based on Pd-Catalyzed C-H Bond Activation.Prog. Chem.2012, 24, 1324-1336.

 9. Wang, Y.; Cheng, G.; Cui, X., Easily Modified Directing Groups for the Palladium-Catalyzed C-H Functionalization. Chinese J. Org. Chem. 2012, 32, 2018-2039. 

[Link]


Before Huaqiao University


8. Cheng, G.; Wang, X.; Zhu, R.; Shao, C.; Xu, J.; Hu, Y., Total Synthesis of (-)-Cocaine and (-)-Ferruginine. J. Org. Chem. 2011, 76, 2694-2700. 

[Link]


7. Cheng, G.; Wang, X.; Su, D.; Liu, H.; Liu, F.; Hu, Y., Preparation of Enantiopure Substituted Piperidines Containing 2-Alkene or 2-Alkyne Chains: Application to Total Syntheses of Natural Quinolizidine-Alkaloids. J. Org. Chem. 2010, 75, 1911-1916.

[Link]


6. Xu, J.; Wang, X.; Shao, C.; Su, D.; Cheng, G.; Hu, Y., Highly Efficient Synthesis of Phenols by Copper-Catalyzed Oxidative Hydroxylation of Arylboronic Acids at Room Temperature in Water. Org. Lett. 2010, 12, 1964-1967

[Link]


5. Shao, C.; Cheng, G.; Su, D.; Xu, J.; Wang, X.; Hu, Y., Copper(I) Acetate: A Structurally Simple but Highly Efficient Dinuclear Catalyst for Copper-Catalyzed Azide-Alkyne Cycloaddition. Adv. Synth. Catal. 2010, 352, 1587-1592.

[Link]


4. Liu, H.; Su, D.; Cheng, G.; Xu, J.; Wang, X.; Hu, Y., Enantiopure 2,6-disubstituted piperidines bearing one alkene- or alkyne-containing substituent: preparation and application to total syntheses of indolizidine-alkaloids. Org. Biom. Chem. 2010, 8, 1899-1904. 

[Link]

                                           

 

3. Xu, J.; Cheng, G.; Su, D.; Liu, Y.; Wang, X.; Hu, Y., Direct ortho-Arylation of N-Phenacylpyridinium Bromide by Palladium-Catalyzed C-H-Bond Activation. Chem-Eur. J. 2009, 15, 13105-13110.

[Link]


 

2. Liu, B.; Su, D.; Cheng, G.; Liu, H.; Wang, X.; Hu, Y., An Efficient Method for the Preparation of Versatile Building Blocks: 1-Substituted 2,2-Dimethoxyethylamine Hydrochlorides. Synthesis 2009, 3227-3232.

[Link]

  

 

 

1. Dai, L. ; Cheng G.; Wang X.; Chen Y., Synthesis of 2-mercapto-5-methoxyimidazo[4,5-b]pyridine. J. Chem. Ind. Eng. (China), 2007, 58, 656-659. 

 


授权专利:

5. 程国林;吕薇薇;一种乙烯基硅\锗\锡烷衍生物的制备方法,ZL201810736263.7

4. 程国林;余佳;一种3'-芳基-2,2'-联吡啶-6-甲酰胺衍生物的制备方法,ZL201810416998.1

3. 程国林;薛露露;一种2,4-二取代吡咯衍生物的制备方法,ZL201711327068.0

2. 程国林, 翁云翔,一种多取代二氢呋喃[2,3-b]吡啶衍生物的制备方法,ZL201710065164.6

1. 程国林, 翁云翔,一种多取代吡啶衍生物的制备方法,CN201710068114.3



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